United States

The coupling between ferroelectric and magnetic orders is an enduring experimental challenge with fundamental importance to elucidate the nature of magnetoelectric (ME) effects in multiferroic materials. In this work, we have studied the response of magnetization to ferroelectric switching in thin-film hexagonal YbFeO3, an improper multiferroic which is a fruitful platform for investigating the ME coupling in single-phase materials. The bulk ME decoupling and potential domain-wall ME coupling were revealed using X-ray magnetic circular dichroism (XMCD) measurements with in-situ ferroelectric polarization switching. Our Landau theory analysis suggests that the bulk ME-coupled ferroelectric switching path has an higher energy barrier than that of the ME-decoupled path; this extra barrier energy is also too high to reduce by the magneto-static energy in the process of breaking single magnetic domains into multi-domains. In addition, the reduction of magnetization around the ferroelectric domain walls predicted by the Landau theory, may induce the domain-wall ME coupling in which he magnetization is correlated with the density of ferroelectric domain walls. These results provide important experimental evidences and theoretical insights to the rich possibilities of ME couplings in hexagonal ferrites.References: 1] J.F. Scott, Room-temperature multiferroic magnetoelectrics, NPG Asia Materials, 5 (2013) e72-e72. [2] S. Fusil, V. Garcia, A. Barthelemy, M. Bibes, Magnetoelectric Devices for Spintronics, Annual Review of Materials Research, 44 (2014) 91-116. [3] P. Mandal, M.J. Pitcher, J. Alaria, H. Niu, P. Borisov, P. Stamenov, J.B. Claridge, M.J. Rosseinsky, Designing switchable polarization and magnetization at room temperature in an oxide, Nature, 525 (2015) 363-366. [4] N.A. Spaldin, R. Ramesh, Advances in magnetoelectric multiferroics, Nat. Mater., 18 (2019) 203-212. [5] S.-W. Cheong, Topological domains/domain walls and broken symmetries in multiferroics, National Science Review, 6 (2015) 624-626. [6] S. Dong, J.M. Liu, S.W. Cheong, Z.F. Ren, Multiferroic materials and magnetoelectric physics: symmetry, entanglement, excitation, and topology, Adv Phys, 64 (2015) 519-626. [7] M. Fiebig, T. Lottermoser, D. Meier, M. Trassin, The evolution of multiferroics, Nature Reviews Materials, 1 (2016). [8] H. Das, A.L. Wysocki, Y. Geng, W. Wu, C.J. Fennie, Bulk magnetoelectricity in the hexagonal manganites and ferrites, Nature communications, 5 (2014) 2998. [9] S. Artyukhin, K.T. Delaney, N.A. Spaldin, M. Mostovoy, Landau theory of topological defects in multiferroic hexagonal manganites, Nat. Mater., 13 (2014) 42-49. [10] W. Wang, J. Zhao, W. Wang, Z. Gai, N. Balke, M. Chi, H.N. Lee, W. Tian, L. Zhu, X. Cheng, D.J. Keavney, J. Yi, T.Z. Ward, P.C. Snijders, H.M. Christen, W. Wu, J. Shen, X. Xu, Room-temperature multiferroic hexagonal LuFeO3 films, Phys Rev Lett, 110 (2013) 237601. [11] X. Xu, W. Wang, Multiferroic hexagonal ferrites (h-RFeO3, R = Y, Dy-Lu): a brief experimental review, Modern Physics Letters B, 28 (2014) 1430008. [12] S. Cao, K. Sinha, X. Zhang, X. Zhang, X. Wang, Y. Yin, A.T. N&#39;Diaye, J. Wang, D.J. Keavney, T.R. Paudel, Y. Liu, X. Cheng, E.Y. Tsymbal, P.A. Dowben, X. Xu, Electronic structure and direct observation of ferrimagnetism in multiferroic hexagonal YbFeO3, Physical Review B, 95 (2017). [13] W. Wang, J.A. Mundy, C.M. Brooks, J.A. Moyer, M.E. Holtz, D.A. Muller, D.G. Schlom, W. Wu, Visualizing weak ferromagnetic domains in multiferroic hexagonal ferrite thin film, Physical Review B, 95 (2017). [14] K. Sinha, H.H. Wang, X. Wang, L.Y. Zhou, Y.W. Yin, W.B. Wang, X.M. Cheng, D.J. Keavney, H.B. Cao, Y.H. Liu, X.F. Wu, X.S. Xu, Tuning the Neel Temperature of Hexagonal Ferrites by Structural Distortion, Phys Rev Lett, 121 (2018). [15] K. Du, B. Gao, Y.Z. Wang, X.H. Xu, J. Kim, R.W. Hu, F.T. Huang, S.W. Cheong, Vortex ferroelectric domains, large-loop weak ferromagnetic domains, and their decoupling in hexagonal (Lu, Sc)FeO3, Npj Quantum Mater, 3 (2018). [16] Y. Geng, N. Lee, Y.J. Choi, S.W. Cheong, W. Wu, Collective magnetism at multiferroic vortex domain walls, Nano Lett, 12 (2012) 6055-6059. [17] J.A. Moyer, R. Misra, J.A. Mundy, C.M. Brooks, J.T. Heron, D.A. Muller, D.G. Schlom, P. Schiffer, Intrinsic magnetic properties of hexagonal LuFeO3 and the effects of nonstoichiometry, APL Materials, 2 (2014) 012106. [18] M.E. Holtz, K. Shayovalov, J.A. Mundy, C.S. Chang, Z.W. Yan, E. Bourret, D.A. Muller, D. Meier, A. Cano, Topological Defects in Hexagonal Manganites: Inner Structure and Emergent Electrostatics, Nano Lett, 17 (2017) 5883-5890. [19] T. Matsumoto, R. Ishikawa, T. Tohei, H. Kimura, Q. Yao, H. Zhao, X. Wang, D. Chen, Z. Cheng, N. Shibata, Y. Ikuhara, Multivariate statistical characterization of charged and uncharged domain walls in multiferroic hexagonal YMnO3 single crystal visualized by a spherical aberration-corrected STEM, Nano Lett, 13 (2013) 4594-4601. [20] Y.K. Jeong, J.H. Lee, S.J. Ahn, S.W. Song, H.M. Jang, H. Choi, J.F. Scott, Structurally tailored hexagonal ferroelectricity and multiferroism in epitaxial YbFeO3 thin-film heterostructures, J Am Chem Soc, 134 (2012) 1450-1453. [21] Y.N. Geng, H. Das, A.L. Wysocki, X.Y. Wang, S.W. Cheong, M. Mostovoy, C.J. Fennie, W.D. Wu, Direct visualization of magnetoelectric domains, Nature materials, 13 (2014) 163-167.

MMM 2020

Magnetoelectric coupling and decoupling in multiferroic hexagonal YbFeO3 thin films

The 65th Annual Conference on Magnetism and Magnetic Materials (MMM 2020) was held in a virtual form. The COVID-19 pandemic, with its associated uncertainty about international travel and the ability to gather in large groups, meant that the Steering Committee decided to cancel the face-to-face meeting that had been planned in Palm Beach, Florida November 2-6, 2020.

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The coupling between ferroelectric and magnetic orders is an enduring experimental challenge with fundamental importance to elucidate the nature of magnetoelectric (ME) effects in multiferroic materials. In this work, we have studied the response of magnetization to ferroelectric switching in thin-film hexagonal YbFeO3, an improper multiferroic which is a fruitful platform for investigating the ME coupling in single-phase materials. The bulk ME decoupling and potential domain-wall ME coupling were revealed using X-ray magnetic circular dichroism (XMCD) measurements with in-situ ferroelectric polarization switching. Our Landau theory analysis suggests that the bulk ME-coupled ferroelectric switching path has an higher energy barrier than that of the ME-decoupled path; this extra barrier energy is also too high to reduce by the magneto-static energy in the process of breaking single magnetic domains into multi-domains. In addition, the reduction of magnetization around the ferroelectric domain walls predicted by the Landau theory, may induce the domain-wall ME coupling in which he magnetization is correlated with the density of ferroelectric domain walls. These results provide important experimental evidences and theoretical insights to the rich possibilities of ME couplings in hexagonal ferrites.References: 1] J.F. Scott, Room-temperature multiferroic magnetoelectrics, NPG Asia Materials, 5 (2013) e72-e72. [2] S. Fusil, V. Garcia, A. Barthelemy, M. Bibes, Magnetoelectric Devices for Spintronics, Annual Review of Materials Research, 44 (2014) 91-116. [3] P. Mandal, M.J. Pitcher, J. Alaria, H. Niu, P. Borisov, P. Stamenov, J.B. Claridge, M.J. Rosseinsky, Designing switchable polarization and magnetization at room temperature in an oxide, Nature, 525 (2015) 363-366. [4] N.A. Spaldin, R. Ramesh, Advances in magnetoelectric multiferroics, Nat. Mater., 18 (2019) 203-212. [5] S.-W. Cheong, Topological domains/domain walls and broken symmetries in multiferroics, National Science Review, 6 (2015) 624-626. [6] S. Dong, J.M. Liu, S.W. Cheong, Z.F. Ren, Multiferroic materials and magnetoelectric physics: symmetry, entanglement, excitation, and topology, Adv Phys, 64 (2015) 519-626. [7] M. Fiebig, T. Lottermoser, D. Meier, M. Trassin, The evolution of multiferroics, Nature Reviews Materials, 1 (2016). [8] H. Das, A.L. Wysocki, Y. Geng, W. Wu, C.J. Fennie, Bulk magnetoelectricity in the hexagonal manganites and ferrites, Nature communications, 5 (2014) 2998. [9] S. Artyukhin, K.T. Delaney, N.A. Spaldin, M. Mostovoy, Landau theory of topological defects in multiferroic hexagonal manganites, Nat. Mater., 13 (2014) 42-49. [10] W. Wang, J. Zhao, W. Wang, Z. Gai, N. Balke, M. Chi, H.N. Lee, W. Tian, L. Zhu, X. Cheng, D.J. Keavney, J. Yi, T.Z. Ward, P.C. Snijders, H.M. Christen, W. Wu, J. Shen, X. Xu, Room-temperature multiferroic hexagonal LuFeO3 films, Phys Rev Lett, 110 (2013) 237601. [11] X. Xu, W. Wang, Multiferroic hexagonal ferrites (h-RFeO3, R = Y, Dy-Lu): a brief experimental review, Modern Physics Letters B, 28 (2014) 1430008. [12] S. Cao, K. Sinha, X. Zhang, X. Zhang, X. Wang, Y. Yin, A.T. N'Diaye, J. Wang, D.J. Keavney, T.R. Paudel, Y. Liu, X. Cheng, E.Y. Tsymbal, P.A. Dowben, X. Xu, Electronic structure and direct observation of ferrimagnetism in multiferroic hexagonal YbFeO3, Physical Review B, 95 (2017). [13] W. Wang, J.A. Mundy, C.M. Brooks, J.A. Moyer, M.E. Holtz, D.A. Muller, D.G. Schlom, W. Wu, Visualizing weak ferromagnetic domains in multiferroic hexagonal ferrite thin film, Physical Review B, 95 (2017). [14] K. Sinha, H.H. Wang, X. Wang, L.Y. Zhou, Y.W. Yin, W.B. Wang, X.M. Cheng, D.J. Keavney, H.B. Cao, Y.H. Liu, X.F. Wu, X.S. Xu, Tuning the Neel Temperature of Hexagonal Ferrites by Structural Distortion, Phys Rev Lett, 121 (2018). [15] K. Du, B. Gao, Y.Z. Wang, X.H. Xu, J. Kim, R.W. Hu, F.T. Huang, S.W. Cheong, Vortex ferroelectric domains, large-loop weak ferromagnetic domains, and their decoupling in hexagonal (Lu, Sc)FeO3, Npj Quantum Mater, 3 (2018). [16] Y. Geng, N. Lee, Y.J. Choi, S.W. Cheong, W. Wu, Collective magnetism at multiferroic vortex domain walls, Nano Lett, 12 (2012) 6055-6059. [17] J.A. Moyer, R. Misra, J.A. Mundy, C.M. Brooks, J.T. Heron, D.A. Muller, D.G. Schlom, P. Schiffer, Intrinsic magnetic properties of hexagonal LuFeO3 and the effects of nonstoichiometry, APL Materials, 2 (2014) 012106. [18] M.E. Holtz, K. Shayovalov, J.A. Mundy, C.S. Chang, Z.W. Yan, E. Bourret, D.A. Muller, D. Meier, A. Cano, Topological Defects in Hexagonal Manganites: Inner Structure and Emergent Electrostatics, Nano Lett, 17 (2017) 5883-5890. [19] T. Matsumoto, R. Ishikawa, T. Tohei, H. Kimura, Q. Yao, H. Zhao, X. Wang, D. Chen, Z. Cheng, N. Shibata, Y. Ikuhara, Multivariate statistical characterization of charged and uncharged domain walls in multiferroic hexagonal YMnO3 single crystal visualized by a spherical aberration-corrected STEM, Nano Lett, 13 (2013) 4594-4601. [20] Y.K. Jeong, J.H. Lee, S.J. Ahn, S.W. Song, H.M. Jang, H. Choi, J.F. Scott, Structurally tailored hexagonal ferroelectricity and multiferroism in epitaxial YbFeO3 thin-film heterostructures, J Am Chem Soc, 134 (2012) 1450-1453. [21] Y.N. Geng, H. Das, A.L. Wysocki, X.Y. Wang, S.W. Cheong, M. Mostovoy, C.J. Fennie, W.D. Wu, Direct visualization of magnetoelectric domains, Nature materials, 13 (2014) 163-167.

poster

An important task in micromagnetics is performing a large ensemble of simulations of a structure with only one or a few changed parameters. An example is computing write error rates in magnetic random-access memories (MRAM), where simulations are needed for different stochastic thermal fields. Such computations, which are done by multiple runs on a single or multiple computing devices. have various numerical overheads related to preprocessing, matrix operations, and excessive data storage. We demonstrate a computational approach for performing a large batch of repetitive micromagnetic simulations on a Graphics Processing Unit (GPU) simultaneously. This batched approach has the following benefits: (i) it utilizes GPUs much more efficiently than the traditional approach of running multiple simulations, including much increased speed and reduced memory consumption, (ii) it hides various numerical overheads, such as preprocessing as well as matrix and time stepping operations, (iii) it makes obtaining results and post-processing much more efficient by allowing computing only required properties, e.g. ensemble averages or switching counts. We extended our FEM based micromagnetic framework FastMag to implement the batched approach in all code components, including pre-processing, matrix operations (Fig. 1a), time stepping with adaptivity to step, order, and decisions of a stopping evens per instance (Fig. 1b). Figure 2 shows major improvements of the computational time and memory consumption for switching simulations of an MRAM cell using three 100-instance batch scenarios on an Nvidia GTX1080 GPU: sequential launching of 100 instances, simulating a 100 x 100 array of sufficiently separated cells (to prevent the strong magnetostatic coupling), batched approach. This work was supported as part of the Quantum Materials for Energy Efficient Neuromorphic Computing, an EFRC funded by the U.S. DOE, Office of Science.

High-performance micromagnetics on GPUs for batched simulations

We introduce flatspin, a novel simulator for artificial spin ices (ASI), i.e., ensembles of dipole coupled nanomagnets arranged in a deliberately constructed geometry. Understanding the complex behavior of these systems has provided insight into a wide range of phenomena [4]. Modeling the dynamics of ASI and their connection to the specific design has been paramount to the progression of ASI research [5]. However, conventional modeling techniques are often either too computationally costly or do not provide enough insight into the dynamics of the ASI. Monte Carlo methods approximating each magnet as a single dipole are useful in the search for low-energy configurations [1, 6], but capturing state transitions and dynamics observed in real systems is challenging. On the other hand, high-fidelity micromagnetic simulations are restricted to a small number of nanomagnets due to the computational cost. With the relatively small systems available through this approach, it is difficult to capture large-scale emergent behavior, e.g. [6]. With flatspin, we offer a different approach to the challenge of modeling, and aim to capture large-scale ASI behaviors. At the heart of flatspin lies a robust magnetic dipole model and a switching criteria based on a generalized Stoner-Wohlfarth model. GPU acceleration together with a model optimized for speed enables flatspin to simulate realistic dynamics of millions of magnets within practical time frames. We demonstrate the versatility of flatspin by modeling a diverse set of established experimental results. Reproduced results include emergent fine-scale patterns in kagome ASI [3], large-scale domain sizes in square ASI [6], and different magnetic ordering of square and pinwheel ASI [2] (see Fig. 1). Furthermore, magnetization details of pinwheel ASI during field-driven reversal have been reproduced, for the first time, by a dipole model. With its capability to model ASI dynamics at unprecedented speeds, we believe flatspin will be an asset to the ASI community.References: [1] X. Ke, J. Li, C. Nisoli et al., Physical Review Letters., Vol. 101(3), p.037205 (2008) [2] R. Macêdo, G. M. Macauley, F. S. Nascimento et al., Physical Review B., Vol. 98(1), p. 014437 (2018) [3] E. Mengotti, L. J. Heyderman, A. F. Rodríguez et al., Nature Physics., Vol. 7(1), p.68 (2011) [4] S. H. Skjærvø, C. H. Marrows, R. L. Stamps et al., Nature Reviews Physics., Vol. 2(1), p.13–28 (2020) [5] R. L. Stamps, Nature Physics., Vol. 10(9), p.623–624 (2014) [6] S. Zhang, I. Gilbert, C. Nisoli, Nature., Vol. 500(7464), p.553–557 (2013)

Introducing Flatspin: Enabling Large Scale Dynamical Artificial Spin Ice Simulations

Droplet solitons are magnetization fluctuations that preserve their shape as they precess with uniform frequency ω=0. They satisfy a delicate balance between anisotropy and exchange interactions, and decay in the presence of dissipation. To prevent this, a spin polarized current σ can be applied via a nanocontact of radius ρ*. The magnitude of the current can be increased to induce switching between uniform precession at the ferromagnetic resonance frequency (ω=1), and a stable precession at a frequency larger than the Zeeman frequency (ω=0, in zero applied field). In the absence of dissipation, conservative solitons of frequency ω0 are described by a function Θ(ρ;ω0), where Θ is the angle of the magnetization with the easy axis and ρ is the distance to the center of the nanocontact1. We introduce an effective energy ξ that quantifies the work done (against damping and spin torque) to create a fluctuation of arbitrary shape Θ(ρ). We show that, for specific values of σ, some conservative soliton solutions are saddles of ξ. This allows us to calculate activation barriers Δξ between uniform precession at the ferromagnetic resonance and stable solitons. We present results of Δξ as a function of σ for a variety of nanocontact radii ρ* and spin-torque anisotropy parameters ν. We present micromagnetic simulations with a modified Spin-Transfer-Torque extension in OOMMF which uses the effective energy ξ introduced here. In this way, the difference of energies between transition states and metastable configurations can be used to estimate annihilation rates of droplet solitons.References: [1] Gabriel D. Chaves-O’Flynn and D. L. Stein, Phys. Rev. B 101, 184421 (2020) [2] M. A. Hoefer, T. J. Silva, and M. W. Keller, Phys. Rev. B 82, 054432 (2010).

Thermal activation barriers for creation and annihilation of magnetic droplet solitons in the presence of spin transfer torque

The magnetodynamic properties of a square thin-film micromagnet (2μm×2μm×16nm) with a flux-closure magnetic ground state were investigated by micromagnetic simulations. The system was excited with an applied magnetic field, displacing the vortex core sufficiently far from its equilibrium position to result in a nonlinear relaxation upon removal of the field. We focus on the edge defects that are created in the process of the vortex core displacement, and carry a half-integer winding number. The edge topological defects are seen to perform quasi-periodic exchange explosions and a resulting emission of short-wavelength spin waves upon travelling back to the equilibrium position. The exchange explosions of the edge topological defects are investigated and explained in terms of vortex/antivortex creation and the formation of a Bloch point. This finding could prove useful to the development of nanoscale devices for periodic generation of high-frequency microwave radiation.References: 1. S. D. Slöetjes, E. Folven, and J. K. Grepstad, Physical Review B Vol. 101, p. 014450 (2020) 2. R. Hertel, and C. M. Schneider, Physical Review Letters Vol. 97, p. 177202 (2006) 3. M. Noske et al., Physical Review B Vol. 91, p. 014414 (2015) 4. S. D. Slöetjes et al., Applied Physics Letters Vol. 112, p. 042401 (2018)

Exchange Explosions of Topological Edge Defects in a Square Micromagnet

Recently, noncollinear antiferromagnets (AFMs) have become one of the most fascinating classes among AFMs, because they exhibit various peculiar magnetotransport properties include the anomalous Hall effect (AHE).[1] The theoretical study shows that the noncollinear AFM Néel vector can be manipulated by spin current with a realistic current density of 107 A/cm2[2]. The antiperovskite manganese nitride Mn3GaN (MGN) is a good platform to investigate the electrical current manipulation of noncollinear AFMs. In MGN, the Mn atoms form a kagome lattice in the (111) plane. The Neel temperature is reported to be above 380 K[3], which are relatively high for this class of materials. In this presentation, we show the spin-torque switching of noncollinear AFM MGN/Pt bilayers at room temperature[4] as well as AHE. MGN (001) films were prepared on MgO (001) substrates by reactive magnetron sputtering. The AHE versus magnetic field curve for MGN films are shown in Fig. 1. The AHE loop is observed with the same coercive field as the out of plane magnetization curves for MGN films. Therefore, the AHE loops shows the electrical detection of the magnetization for MGN films. The change in the Hall resistivity as a function of current density for MGN(20 nm)/Pt(3 nm) bilayers is shown in Fig. 2. Hall resistivity changes sharply and a clear hysteresis loop is observed at 300 K without an external magnetic field. The change of Hall resistivity is the same as AHE loop shown in Fig. 1, indicating the electrical write–read operation of noncollinear AFM Néel vector. The critical current density is estimated to be 3.6×106 A/cm2, which is one to two orders of magnitude smaller than that for typical FM/HM bilayers[5] and the threshold current for collinear AFMs NiO/Pt spin-torque switching.[6] These results open the pathway to the efficient control of the noncollinear AFM order.References: [1] S. Nakatsuji, N. Kiyohara, and T.Higo, Nature 527, 212-215(2015). [2] Y. Yamane, O. Gomonay, and J. Sinova, Phys. Rev. B 100, 054415 (2019). [3] W. J. Feng, D. Li, Y. F. Dend, and Q. Zhang et al., J. Mater. Sci. 45, 2770 (2010). [4] T. Hajiri, S. Ishino, and K. Matsuura et al., Appl. Phys. Lett. 115, 052403 (2019). [5] L. Liu, O. J. Lee, and T. J. Gudmundsen et al., Phys. Rev. Lett. 109, 096602 (2012). [6] X. Z. Chen, R. Zarzuela, and J. Zhang et al., Phys. Rev. Lett. 120, 207204 (2018).

Electrical switching of Hall resistance in noncollinear antiferromagnetic antiperovskite nitrides

Antiferromagnets (AFMs) are promising spintronic materials compared to ferromagnets, since they potentially enable faster operation, enhanced stability with respect to interfering magnetic fields and higher bit packing density due to the absence of stray fields [1]. However, the use of AFMs in applications requires efficient electrical reading and writing of information. While current-induced switching in NiO/Pt thin film systems has been shown, with various mechanisms proposed [2-4], key information such as the absolute torque strength is missing. Studying MgO//CoO(001)/Pt entails a number of advantages: due to the compressive strain by the substrate, a fourfold in-plane magnetic anisotropy of the CoO layer with two easy axes in the (001) plane is favored and the spin flop field is accessible [5]. Such anisotropy is ideal for applications where the orientation of the Néel order n is read by spin Hall magnetoresistance (SMR) [6,7]. To study current-induced switching, we used 8-arms Hall stars devices with the pulsing arms oriented along the [110] and [-110] easy axes directions (Fig. 1a). Initially n is aligned along [110]. When current pulses are applied along the contacts 3-2 (initial state n ‖ jpulse), the transverse resistance drops after the first pulse, indicating a current-induced 90° n rotation (Fig. 1b). Performing a MR scan with field along 4-1 afterwards (Fig. 1c) yields a field-induced spin flop transition of n back to the initial state (Fig. 1d). By applying current pulses and magnetic fields, we can quantify the current field equivalence of the current-induced torques on the reorientation of n in the CoO, showing that, for the switching of AFMS, currents are much more efficient than magnetic fields.References: [1] V. Baltz et al., Rev. Mod. Phys., 90, 015005 (2018). [2] X. Z. Chen et al., PRL, 120, 207204 (2018). [3] L. Baldrati et al., PRL, 123, 177201 (2019). [4] P. Zhang et al., PRL 123, 247206 (2019). [5] L. Baldrati et al., ArXiv:2003.05923 (2020). [6] H. Nakayama et al., PRL, 110, 206601 (2013). [7] L. Baldrati et al., PRB, 98, 024422 (2018).

Quantifying current-induced torques leading to Néel vector switching in CoO/Pt bilayers

We predict staggered-field-stabilized collinear, spiral, cone, skrymion crystal (SkX), and square crystal (SC) of vortices and antivortices phases in antiferromagnets (see figure). In SkX and SC phases, magnons experience emergent gauge fields, which leads to magnon-mediated topological spin responses. The underlying physics can be qualitatively understood by considering magnon Landau levels induced by the fictitious magnetic flux. In the long wavelength limit, the unevenly spaced energy bands can be described by the relativistic Klein-Gordon equation. As we propose, these Landau levels can be also realized in antiferromagnetic magnonic topological insulator where the fictitious flux is induced by inhomogeneous DMI. A smoking gun experiment observing the Hofstadter's butterfly of magnons in AFM could establish the connection between emergent electromagnetism and topological properties of antiferromagnetic magnons.

Magnon Landau Levels and Topological Spin Responses in Antiferromagnets

We present a spin-transfer torque oscillator (STO) based on composite (hard-soft) synthetic antiferromagnets (CSAFs) with perpendicular uniaxial magnetic anisotropy energy density. The CSAF STO can operate with and without an applied field and generates strong oscillations in a broad frequency range from tens to hundreds GHz with precessions mostly generated by the soft layer. The STO is comprises of a cylindrical cross – section stack of diameter D (Fig.1), including a reference layer and a free layer composed of SAF layers (FLsoft and FLhard). FLhard is much harder than FLsoft and the sub-layers are exchange coupled with surface exchange energy density JAF. The results are obtained via micromagnetic simulations with the FastMag1 simulator. Fig.1 shows the precession frequency of the FLsoft as a function of the applied current density J for weak and strong JAF. The precession frequency of FLsoft is proportional to JAF and J and it can be tuned in a broad range of frequencies up to 200 GHz. Fig.2 shows the time dependence of the magnetization components for FLsoft and FLhard. Both z-components are in the same direction while the in-plane components are opposite. The precession direction sense is clockwise for both layers, but the precession is dominated by the soft layer, i.e. the device generates a strong oscillating magnetic field. The operation mechanism is based on the exchange field due to the AF coupling, which is similar to AF STO2. However, CSAF STO offers a great flexibility in tuning the parameters and practicality in the material choice. It can be used to generate electric signal or for microwave assisted magnetic recording, This work was supported by the Quantum-Materials for Energy Efficient Neuromorphic-Computing(Q-MEEN-C), an Energy Frontier Research Center funded by the U.S. DOE, under Award No. DE-SC0019273.References: [1] R. Chang, S. Li, M. V. Lubarda, B. Livshitz, and V. Lomakin, J Appl Phys 109 (3), 07D358 (2011). [2] V. Puliafito, R. Khymyn, M. Carpentieri, B. Azzerboni,1 V. Tiberkevich, A. Slavin, and G. Finocchio, PRB 99, 024405 (2019).

Spin-transfer torque oscillator based on composite synthetic antiferromagnets

Bayesian optimization (BO) is a well-developed machine learning algorithm for black box optimization. In BO a predictive model, here a Gaussian process regression, is implemented to predict the black box function and the uncertainty of the predictive model is evaluated as predicted variance, then an acquisition function defined by the surrogate predictive model decides where to sample next. In this study we applied this technique to known ferroic materials such as ferromagnetic (Fe100−y Gay)1−xBx (x=0–21 & y=9–17) and ferromagnetic (Co0.5Fe0.5)1-xCx (x=0–16) to provide proof of concept of how BO can be used to optimize properties such as magnetostriction and ferromagnetic resonance (FMR) linewidth with fewer samples required than traditional experimental approaches.1,2 Additionally, we applied this technique to optimize thin films of ferromagnetic (Fe100−y Gay)1−xCx (x=1–26 and y=2–18) and ferroelectric (HfO2)1-xYx (x=0–15). For each of these systems, we applied BO through building a predictive model with the GPy library (https://sheffieldml.github.io/GPy/) and evaluating the next experiment to sample with the GPyOpt library (https://github.com/SheffieldML/GPyOpt), both in python.References: [1] J. Lou et al. Appl. Phys. Lett. 91, 182504 (2007). [2] J. Wang et al. Phys. Rev. Applied 12, 034011 (2019)

Application of Bayesian Optimization to Ferroic Materials Development

The BaTiO3 (BTO)/CoFe multiferroic material interface is an example of an interface which displays voltage-controlled magnetic anisotropy (VCMA), a valuable property in the operation of multiferroic tunnel junctions in an STT-MRAM device. Through first principles calculations, it is possible to predict trends in film magnetic anisotropy energy (MAE) and enumerate the individual physical mechanisms contributing to ferroelectric control of MAE in the CoFe film. For CoFe of up to 2 atomic layers on BTO, MAE can be modulated by ferroelectric switching through Fe-O orbital interations in BaO-terminated interfaces, and Ti-Fe orbital interactions in TiO2-terminated interfaces. A difference in interface termination produces a difference of MAE in CoFe films of up to 9 atomic layers. The inclusion of a 5d transition metal capping layer (Hf, Ta, W, Re, Os, Ir, Pt, or Au) on top of the CoFe layer exerts a significant effect on both MAE and the ferroelectric switching effect, in particular inducing a discernible ferroelectric switching control even in thicker CoFe films. This points to the additional, if counterintuitive, contribution of CoFe 3d top interface (or surface) states and their interactions with partially filled 5d orbitals of the capping layer atoms.References: A. P. Chen and Y. P. Feng, ACS Appl. Mater. Interfaces., Vol. 12, p25383-25389 (2020) A. P. Chen, W. Lin, J.-S. Chen, and Y. P. Feng, in preparation.

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