United States

Ultrafast generation of chiral magnetic order is one of the most sought-after technology for its potential application in next generation magnetic memory devices [1]. Recent experimental demonstration of generation of skyrmions with ultrafast laser pulses [2] has opened new horizons regarding the experimental feasibility of achieving this. In spite of such immense experimental achievement, the theoretical understanding of the underlying physics is still not very clear. Most of the existing studies tries to explain this with classical magnetisation dynamics only and thus completely miss the impact of the electronic interactions which plays crucial role in early sub-picosecond regime. More advanced TD-DFT based approaches are quite successful in explaining the fast dynamics in this regime, however, they are not quite fruitful in explaining the slow magnetisation dynamics which can last for several picoseconds. In this presentation we bridge this gap with the help of a quantum-classical hybrid approach which allows us to reveal the physics with a sub-femtosecond resolution and at the same time look at the steady state after several picoseconds [3]. We have successfully identified both the inherent and emergent interactions which drives the intertwined electronic and magnetic interaction leading to a stable chiral configuration and thus can predict their lifetime as well. We show here that the laser assisted dynamics is inherently different from the predictions of phenomenological two/three temperature model which has been widely used in modelling ultrafast demagnetisation. We show that the thermal re-population leads to formation of multiple domains with higher energy and less stability compared to smooth spiral formed by laser excitation. The final chiral configuration can be tuned both with laser and material parameters and formation can sustain at moderate temperature which makes our findings feasible for experimental realisation and thus would be instrumental in revealing the rich physics of ultrafast optical manipulation of the magnetisation.

![](https://assets.underline.io/uploads/markdown_image/1/image/17b5b1fc1f24b7f50457de2d6090ae8f.jpg)

Comparison of magnetisation dynamics excited by laser and thermal repopulation. Thermal excitation forms multiple domain where laser forms a smooth spiral configuration.

2022 Joint MMM-INTERMAG

Imprinting chirality in collinear magnet with ultrafast laser

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INTERMAG 2021

technical paper

The 15th Joint MMM-INTERMAG Conference (2022 Joint) is sponsored jointly by AIP Publishing and the IEEE Magnetics Society. Members of the international scientific and engineering communities interested in recent developments in fundamental and applied magnetism are invited to attend and contribute to the technical sessions. The technical program will include invited and contributed papers in oral and poster sessions, invited symposia, a plenary session, and an evening session, with about 1500 presentations overall. This Conference provides an outstanding opportunity for worldwide participants to meet their colleagues and collaborators and discuss developments in all areas of magnetism research.

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Advancing the understanding of magnetic relaxation, often discussed in terms of “damping,” is essential for energy-efficient spintronic memories, oscillators, and spin-wave circuits. BCC Fe is an elemental ferromagnet with attractive properties for these applications. Here, we examine magnetic relaxation – i.e., intrinsic and extrinsic damping – in two series of sputter-grown, polycrystalline Fe thin films with distinct structural properties: (1) strongly textured, smooth Fe films grown on Cu and (2) weakly textured, rough Fe films grown on Ag. Out-of-plane ferromagnetic resonance (FMR) measurements reveal intrinsic Gilbert damping parameters of ≈ 0.0024 for all Fe films thicker than 4 nm, regardless of their structural properties, as shown in Fig. 1. This damping parameter range is in quantitative agreement with that for epitaxial Fe [1]. The remarkable invariance with microstructure strongly suggests that intrinsic Gilbert damping is a local property, averaged over a short length scale of a few nm, with limited impact from grain boundaries and film roughness. The in-plane FMR linewidths of the Fe films exhibit pronounced nonlinear frequency dependencies, indicating the presence of strong extrinsic damping. Figure 2 shows the extrinsic linewidth obtained by subtracting the intrinsic Gilbert contribution ΔHG (isotropic for Fe [1,2]) from the total in-plane linewidth ΔHIP. To fit our experimental data, we have used a grain-to-grain two-magnon scattering model [3-5] with two types of correlation functions proposed for modeling self-affine and mounded surfaces [6], which capture inhomogeneities in the film. However, neither of the two correlation functions is able to reproduce the data quantitatively. Our finding points to the need to further examine the fundamental impact of film microstructure on extrinsic damping.

![](https://assets.underline.io/uploads/markdown_image/1/image/1036e2b51a2ec70732f50783b672e744.jpg)


Fig. 1. Out-of-plane Gilbert damping αOOP as a function of film thickness.

![](https://assets.underline.io/uploads/markdown_image/1/image/0dd999a01cf02f7a52d306323d0872e3.jpg)


Fig. 2. In-plane extrinsic FMR linewidth vs frequency for (a) Cu/Fe (8 nm) film and (b) Ag/Fe (25 nm) film. Black squares represent experimental linewidth data. Dashed blue and solid red curves represent the fitted curves using correlation functions proposed for modeling self-affine and mounded surfaces, respectively.

Intrinsic and Extrinsic Damping in Polycrystalline Fe Thin Films

Spin transport across interfaces is fundamental to many spintronic devices. To fully exploit interfacial phenomena, such as spin-orbit torques and spin-pumping, in ferromagnetic (FM) and heavy metal systems (HM) the properties of both the HM layer and the interface must be considered, particularly in the case of perpendicularly magnetised systems [1]. Previously we showed the evolution of spin transport as a function of FM and HM thicknesses [2] and the role of insulating layers [3]. Debates remains regarding the physical basis of interfacial spin transport and the role of proximity polarisation of the HM layer [4]. A notional ‘spin memory loss’ term is often used to represent an interfacial contribution, while for Pt in particular, a magnetic polarisation arises in proximity (PIM) to a ferromagnetic material, opens a question about the role that PIM has upon interfacial spin phenomena, with contradictory reports that it has either a profound effect [5] or no effect [6] on spin transport. Here we present the results of a detailed systematic spin transport and PIM study in the same FM/HM samples. Structures with either a constant Pt thickness and a spacer layer thickness wedge, or a constant spacer layer and a Pt wedge were deposited. A combination of dynamic and static magnetic measurements, along with element specific resonant x-ray measurements at the APS, Argonne Lab, were used to address both the interfacial scattering contribution and the role of PIM in Pt on spin transport and to determine their relative contributions. Figs. 1 and 2 show damping and PIM data, with a persisting Pt moment with a 3nm Au layer, and a clear trend observed between the PIM and dynamic behaviour. These results highlight the role of the d-d orbital hybridisation and the induced moment for efficient interfacial transport, which is key for many spintronic applications.

![](https://assets.underline.io/uploads/markdown_image/1/image/ca60624dc0cead773db990e20080f85b.jpg)

Fig 1: Measured XMCD as a function of Au spacer thickness at both the Pt (blue) and Au (orange) L3 edges for NiFe (7 nm)/ Au / Pt (4 nm)

![](https://assets.underline.io/uploads/markdown_image/1/image/f3928c773ef3592e934476655f51d0ce.jpg)

Fig 2: Damping and Pt XMCD for CoFe/Au/Pt and NiFe/Au/Pt. Dotted lines indicate bulk damping contributions.

The role of proximity induced magnetism on spin transport in multilayered systems

Spin-Hall nano oscillators (SHNOs) [1-4] have recently emerged as an alternative for microwave signal generation and bio-inspired oscillatory computing [3,4]. However, the ferromagnetic layer of the SHNO comes with drawbacks: (a) need for strong external magnetic fields, and (b) limited operational frequencies. As a solution, compensated ferrimagnets provide an alternative as they combine the ultrafast magnetization dynamics of antiferromagnets with a ferromagnet-like spin-orbit-torque (SOT) behavior. For use in SHNOs, it is however important to ensure that such films retain their ferrimagnetic behavior also in ultrathin films. In this work, ferrimagnetic Gdx(FeCo)1-x thin films were grown using co-sputtering of Gd and Fe87.5Co12.5 on high resistance (HR) Si (100) substrates, and their magneto-dynamics was studied using ferromagnetic resonance measurements at room temperature. By tuning the stoichiometry of Gdx(FeCo)1-x films, a nearly compensated behavior is for the first time demonstrated in 2nm thin film (Fig. 1). Values for the effective magnetization and effective Gilbert damping constant (α) of 0.02 Tesla and 0.0078±0.0002 are obtained for 2nm Gd24.4(FeCo)75.6 film, where α is comparable to the lowest value obtained in thick films [5]. The vertical red and yellow lines in Fig. 1(c) show literature values [5,6] for the spin angular momentum (xa) and magnetic momentum (xm) compensation points in thick films. The stoichiometry for the magnetic moment compensation in this work is very close to those [Fig. 1(c)]. In search of high-frequency auto-oscillations in SHNOs, constrictions with 50-300 nm widths were also prepared using Gdx(FeCo)1-x (2-10nm)/Pt(5nm) based stacks and promising results using Brillouin Light Scattering show SOT controllable ferromagnetic modes in these devices.

![](https://assets.underline.io/uploads/markdown_image/1/image/9abf7a526aa9ca9c52175f16a9ed7bff.png)

Fig. 1. (a) Frequency (f) vs. resonance field and (b) Resonance linewidth vs f, of 2 nm thick Gdx(FeCo)1−x films, with x the Gd atomic %. (c) Effective magnetization and effective Gilbert damping constant vs. composition of 2 nm Gdx(FeCo)1−x films; solid symbols represent values obtained by fitting the experimental data to the Kittel’s equation [7] and equation (10) in reference [8], while solid lines are a guide to the eye.

Ultrathin ferrimagnetic GdFeCo films with very low damping

We present an overview of new techniques that can probe the properties of magnetic materials on very short time scales. We present a pump-probe spectroscopy method utilizing tabletop extreme UV (EUV) light produced by high harmonic generation. This EUV source allows us to spectroscopically probe ferromagnetism with multi-element specificity and a time resolution on the order of a few-femtoseconds. This made it possible to uncover that surprisingly, it is possible to excite the spin system in pure ferromagnets and alloys on few-femtosecond time scales [1,2]. With the implementation of a flux monitoring reference arm, we are able to remove source instability and improve data quality while reducing acquisition times.

New Techniques for Probing the Dynamic Properties of Magnetic Materials

Recently, it has been theoretically and experimentally demonstrated that the effects of inertia of magnetization should be considered in the full description of spin dynamics at pico- and femtosecond timescales [1-8]. The nutation motion of magnetization is a manifestation of inertia of the magnetic moments. A rigorous derivation including inertia in the Landau-Lifshitz-Gilbert equation was carried out by Mondal et al. in the Dirac-Kohn-Sham framework [6,7]. Here, we show that inertia effect in magnetization dynamics results in a new type of spin waves, i.e. nutation surface spin waves, which propagate at terahertz frequencies in in-plane magnetized ferromagnetic thin films. Considering the magnetostatic limit, i.e. neglecting exchange coupling, we calculate dispersion relation. In addition, we find that the nutation surface spin waves are backward spin waves [1]. The phase shift between precessing magnetic moments propagates as a spin wave through the ferromagnet because of dipole-dipole or exchange coupling (Fig. 1(a)). Magnetic inertia effects, which are expected to contribute to dynamics of spin waves, originate from spin-orbit coupling. We find that when taking inertia into account one finds that the deviation of alignment of localized moments will propagate through the spin system in the form of both precession and nutation motions, i.e. in ferromagnetic materials one needs to add to all “conventional” spin wave modes a high frequency wave-like motion with small amplitude caused by inertia. Moreover, a different type of waves having predominantly inertial nature appears in ferromagnetic thin films, which we call here nutation surface spin waves. Since these waves have terahertz frequencies (compared to typically GHz frequencies of other spin wave modes), they can be plotted as a small deviation on top of a “frozen” precession motion (Fig. 1(b)).

![](https://assets.underline.io/uploads/markdown_image/1/image/e702e12d86e64bbc071819e5db941fcf.jpg)

Fig. 1. (a) The precession spin wave without inertia (red curve). The blue arrow indicates the motion of the magnetization M. (b) The nutation surface spin wave (purple curve) with a frequency considerably higher than in (a) plotted with small blue circles on top of the “frozen” precession motion.

Dispersion Relation of Nutation Surface Spin Waves in Ferromagnets

In magnetic thin films, large excitation amplitudes can lead to the onset of the first order Suhl instability, where the driven uniform mode undergoes three magnon scattering to two modes of half the frequency and equal and opposite wavevectors. Although experimental studies of the steady-state behavior are established, a comprehensive study of the nonequilibrium behavior over a large range of excitation powers is lacking. We have developed an experimental technique for sensitive detection of the time evolution of the FMR amplitude over five orders of magnitude in power, which provides a highly comprehensive understanding of the three-magnon scattering process. Applying this technique to patterned 3μm thick YIG thin films, we observe strong agreement with our results from micromagnetic simulations of the Suhl instability. We have developed a semianalytical model to explain the three magnon scattering process. This model shows quantitative agreement with experiment and simulation, including a predicted additional regime corresponding to power-dependent nonlinear oscillatory behavior on the order of 50 MHz. Additional observed effects will also be discussed. This work was supported by SMART, a center funded by nCORE, a SRC program sponsored by NIST, DARPA under Grant W911NF-17-0100, MINT at Minnesota, and the NSF XSEDE through Allocation No. TG-ECS200001. We acknowledge the use of MSI resources.

![](https://assets.underline.io/uploads/markdown_image/1/image/1206326856094257491a60e9c5fd8367.jpg)

Time-resolved Nonlinear Magnetization Dynamics in YIG Thin Films

Time-resolved Nonlinear Magnetization Dynamics in YIG Thin Films

One current goal of spintronics is the development of sustainable information technology based on pure spin currents. One promising way to do this is to use spin waves (SWs) in low damping insulating ferrimagnets like yttrium iron garnet (YIG) where relaxation can be controlled by spin orbit torque (SOT) at a heavy metal interface [1]. However, such metal/insulator hybrid devices exhibit saturation of SW amplification due to nonlinear coupling between modes [2]. Two strategies can be considered to overcome these issues. i) Nanopatterning leads to quantization of SW modes [3], thereby limiting the available nonlinear processes [4]. ii) Tuning the perpendicular magnetic anisotropy (PMA) can be used to control the sign of the nonlinear frequency shift [5]. Recently, the growth of ultra-thin films of bismuth doped YIG (BiYIG) with tunable PMA has been achieved [6], resulting in greatly improved characteristics of SOT emitted SWs [7]. Here, we study the magnetization dynamics in individual nanodisks patterned from such a 30 nm thick BiYIG film with submicron diameters. The static magnetic field is perpendicular to the plane. The in-plane microwave field is produced by an integrated antenna. To detect the FMR, we employ a magnetic resonance force microscope [8]. For the largest disks, the amplitude of the FMR peak quickly saturates as the excitation power is increased, which is accompanied by a strong distortion of the absorption line, that broadens and splits into several peaks (Fig1a). Micromagnetic simulations accurately reproduce these features and reveal that a dynamic instability is responsible for the observed behavior. To experimentally probe this complex dynamics, we apply a second, much weaker excitation field of varying frequency, in addition to the main driving field at high power. The frequency modulation spectrum obtained (Fig1b) reflects the existence of rich low-frequency temporal variations in the magnetization dynamics.

![](https://assets.underline.io/uploads/markdown_image/1/image/0f9922ccb39360e331cfbc33deb7fa05.jpg)

Fig 1. (a) Resonance line in the deeply nonlinear regime. (b) Two-tone spectroscopy performed inside the instability region, at μ0Hz = 165 mT.

Dynamic instabilitiy in high power FMR of BiYIG nanodisks

An interesting phenomenon occurs in submicron, magnetic vortex ground state particles as their thickness is increased, and the vortex becomes a fully-fledged three dimensional object. Although the ground state remains largely homogeneous through the thickness, one but needs to apply the smallest of excitation to see the emergent shearing of the magnetization texture and resonant modes associated with it [1,2]. Using the nanostencil fabrication technique[3] we obtained planar arrays of increasingly thick (up to 350 nm) magnetic particles, going beyond thicknesses studied previously. Not only do we observe the inversion of intensities of the modes, as high order modes become the most intense, we see also the complete disappearance of the homogeneous G0 mode, which marks a transition where the 2D dynamic solutions completely cease their existence, see the spectrum presented on Fig. 1. This new effect also goes toward a significant increase of the speed of dynamics in the system. In the course of study we place a special emphasis on taking the real, dome-like particle profiles into account, which, as we show, influence the spectra for thick particles significantly. The profiles used were attained with a help of atomic force microscopy. The realistic boundaries primarily tune the non-radiative standing spin wave modes[4] which in turn affect gyrational modes through hybridization. We observe this through the detailed, microscopic study of mode distributions such as the one on Fig. 2, by matching experimental spectra, and juxtaposing stationary trajectories (in the time domain).

![](https://assets.underline.io/uploads/markdown_image/1/image/8f782616bbfa5a82e7cffe9fbfba735f.jpg)

![](https://assets.underline.io/uploads/markdown_image/1/image/fc47f4d3547c1babcc525b8c1162cc50.jpg)

High Order Gyromode Observation in Dome-like Nanoparticles

High Order Gyromode Observation in Dome-like Nanoparticles

All Optical Helicity Independent Switching (AO-HIS) of magnetization, using single femtosecond laser pulses, has been demonstrated in GdFeCo ferrimagnetic alloys for various concentrations [1] as well as in other structures with antiferromagnetic coupling, Gd/Co, [Tb/Co]n/Ta/CoFeB and Mn2RuxGa [2,3,4]. Up to now, AO-HIS has never been observed for ferromagnetic layers. However, it was shown that a single pulse magnetization reversal of a ferromagnet could be observed in a spin-valve structure [5]. The switching is then achieved by the ultrashort spin current pulse generated from the ultrafast demagnetization of GdFeCo [5,6]. In this work, we study Gdx(FeCo)1-x/Cu/FM spin-valve structures, where FM can be different ferromagnetic layers [7] and the composition x of the GdFeCo alloy is also changed [8]. By increasing the Gadolinium concentration x, we aim at increasing the spin current injected in the copper layer [6]. We show that this can reduce the laser fluence threshold required to observe the FM magnetization reversal. In particular, no AO-HIS of the GdFeCo layer is required and the threshold fluence for the FM layer is around 1.6 mJ/cm2 i.e. comparable to GdFeCo and Gd/Co multilayers [1,2] and smaller than what is achieved for Tb/Co/CoFeB [2] and Mn2RuxGa [3]. We also show that by changing the Curie temperature, the laser pulse duration and the Cu/FM interface, one can control the interaction between the spin current and the FM layer and so the laser fluence threshold. Finally, we measured the dynamics of the reversal of the FM layer, which happens in around a picosecond. We show a model, based on a recent theory for the ultrafast magnetization dynamics of ferromagnets [9], that explains this behavior. We thus designed spin-valve structures that could provide technological advantages regarding both speed and energy efficiency of data storage.

Ultrafast Single Pulse All Optical Magnetization Switching of Ferromagnets

Graphene/ferromagnet interfaces have exhibited various unusual spin-orbit coupling(SOC) related effects despite very small SOC strength of graphene[1-3]. Here we have investigated femtosecond laser induced spin dynamics using an all-optical time-resolved magneto-optical Kerr effect(TR-MOKE) magnetometry in sputter-deposited CoFeB thin films on chemical-vapor-deposition grown single-layer graphene(SLG) by varying the thickness of CoFeB from 1.5 to 6 nm[4]. The ultrafast demagnetization time(τm) extracted using three-temperature modelling(Fig. 1(a)) show a monotonic variation with CoFeB thickness(Fig. 1(b)). The Gilbert damping parameter(α) is directly extracted from the decaying amplitude of precessional oscillation(Fig. 1(c)). We have modelled the CoFeB-thickness-dependent α to estimate the effective spin-mixing conductance(Geff) and two-magnon scattering coefficient(βTMS) for SLG/CoFeB interface(Fig. 1(d)) which revealed spin pumping(SP) [4] as the dominant contributor to modulation of α(Fig. 1(e)). Furthermore, we have observed an inverse relationship between τm and α for SLG/CoFeB heterostructures(Fig. 1(f)) due to the dominance of SP-induced nonlocal spin-transport mechanism[4]. To disentangle other possible interface contributions to the damping such as spin memory loss(SML), we have inserted a 1-nm-thick Cu spacer layer between the SLG and CoFeB. Negligible damping modulation by the insertion of Cu spacer between SLG and CoFeB confirms that additional effects like SML are absent in our system. In summary, this study has provided a qualitative understanding of different ultrafast spin manipulation mechanisms in a graphene-based heterostructure, which can lead towards the next-generation graphene-based ultrafast spintronics devices. AB acknowledges the financial assistance from S. N. Bose National Centre for Basic Sciences(SNBNCBS), India under Project SNB/AB/11-12/96 and SNB/AB/18-19/211. SNP, SM, SC and ArB acknowledge SNBNCBS for respective fellowship.

![](https://assets.underline.io/uploads/markdown_image/1/image/2365a212e2a849241df3b94e8286c456.jpg)

Fig. 1(a) Ultrafast demagnetization in SLG/CoFeB(d) (b) Evolution of τm with d (c) Precessional oscillations at H=3.59 kOe (d) Evolution of α fitted with a phenomenological model (e) Variation of 1/τm as a function of α (f) Contributions of SP and TMS to α.

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